First Observation of Excited States in 226U

First Observation of Excited States in 226U

Octupole Deformation

   Many of the nuclei that we know of are non-spherical, or deformed. In many cases, it is possible to understand the rotational band structures that we observe in terms of a rotating spheroidal shaped nucleus. Since these nuclei are symmetric under reflection, the members of the rotational band will all have the same parity. The observation of low-lying negative-parity states in the 1950's led to the suggestion that some nuclei may possess shapes which are asymmetric under reflection, or pear-shaped.

   The strength of the octupole interaction can be inferred from the spectra that we observe. The figure below shows some of the possiblities.

Octupole Deformation

Experimental Spectra and Level Scheme

   The two figures below show spectra obtained using the JUROSPHERE Ge detector array and the RITU gas-filled recoil separator. The upper figure is the spectrum obtained from the RITU focal plane Si-strip detector. The broad distribution to the left corresponds to the implantation of fusion-evaporation residues from the 22Ne + 208Pb reaction at a bombarding energy of 112 MeV. The peaks at around 7.5 MeV correspond to the subsequent decay of the implanted recoils.

RITU Si-Strip Detector Spectrum

   The lower figure shows rays which occurred in coincidence with recoils followed by an decay of energy 7.57 MeV, within a time interval of 800 ms after the recoil implant. This corresponds to the characteristic decay of 226U.

Gammas from decay of 226U

   The figure above shows the level scheme obtained through energy sum and intensity balance arguments from the -ray spectrum. The figures in brackets are the total transition intensities normalised to that of the 4+ to 2+ transition. Note the similarity to the intermediate case in the potential energy figure, and the reduction in parity splitting with increasing spin.

Alignment Properties

alignment plot for N=134 isotones

   The figure above shows the difference in experimental aligned angular momentum, ix = ix- - ix+, between the negative- and positive- parity bands as a function of rotational frequency, , for the N = 134 isotones: 226U, 224Th, 222Ra and 220Rn. It can be seen from this plot that the behaviour of ix for 226U follows closely that of 224Th and 222Ra, nuclei which are considered to be octupole deformed, like the intermediate case in the potential energy figure. At low values of , ix has a value of approximately 1.5 and tends towards zero with increasing rotational frequency, this can intrepreted as evidence for the enhancement of octupole strength with rotation. At higher rotational frequency, the pairing correlations are weaker, which increases the moment of inertia. Also, the degree of octupole mixing is increased as the single particle states of opposite parity approach each other. This behaviour is in contrast to that of 220Rn, where ix maintains a value of approximately 3 over the full frequency range, due to the rapid alignment of an octupole phonon coupled to the ground-state band. Hence 220Rn is considered to octupole vibrational in nature, more like the nucleus to the left in the potential energy figure.


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Last modified: 6 February 1998
Written by Paul Greenlees, ptg@ns.ph.liv.ac.uk